ACS Catalysis
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AUTHOR INFORMATION
Corresponding Author
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* Email: stn@northwestern.edu; Fax: +1 847ꢀ491ꢀ7713; Tel: + 1
847ꢀ467ꢀ3347.
* Email: frank.tsung@bc.edu; Fax: +1 617ꢀ552ꢀ2321; Tel: + 1
617ꢀ552ꢀ8927.
Author Contributions
The manuscript was written through contributions of all authors.
All authors have given approval to the final version of the manuꢀ
script.
ACKNOWLEDGMENT
This work was supported by the Chemical Sciences, Geosciences,
and Biosciences Division, US Department of Energy through a
grant (DE FG02ꢀ03ꢀER154757) to the Institute of Catalysis for
Energy Processes (ICEP) at Northwestern University (assisꢀ
tantship for R.L.). R.L. additionally acknowledges Sigma Xi for a
GrantsꢀinꢀAid of Research (GIAR) award and support from
Northwestern University as a teaching fellow. S.T.N. acknowlꢀ
edges support from DTRA (HDTRA1ꢀ14ꢀ1ꢀ0014). L.ꢀY.C., A.Y.,
and C.ꢀK.T. acknowledge support from the NSF (CHE 1566445).
This work made use of the Clean Catalysis Facility of Northwestꢀ
ern University Center for Catalysis and Surface Science, which
acknowledges funding from the Department of Energy (DEꢀ
SC0001329) used for the purchase of the Parr reactor units. Exꢀ
perimental facilities at the Integrated Molecular Structure Educaꢀ
tion and Research Center (IMSERC), the Materials Research Cenꢀ
ter (J. B. Cohen XꢀRay Diffraction Facility), and the Northwestꢀ
ern University Atomicꢀ and Nanoscale Characterization Experiꢀ
mental (NUANCE) Center (EPIC and Keck II facilities) at Northꢀ
western University are supported by the Soft and Hybrid Nanoꢀ
technology Experimental (SHyNE) Resource (NSF NNCIꢀ
1542205); the MRSEC program (NSF DMRꢀ1121262) at the
Materials Research Center; the International Institute for Nanoꢀ
technology (IIN, partially supported by the NSF NSEC program,
NSF EECꢀ0647560); the Keck Foundation; and the State of Illiꢀ
nois (through the IIN). ICPꢀOES analyses were carried out at the
Quantitative Bioꢀelement imaging center (QBIC) at NU. We
thank Prof. Mercouri Kanatzidis for the use of the adsorption
instrument and Prof. Justin Notestein for the use of the GCꢀMS
equipment.
ABBREVIATIONS
MOF, metalꢀorganic frameworks; BET, Brunauer–Emmett–
Teller; PXRD, powder Xꢀray diffraction; ICPꢀOES, inductively
coupled plasma optical emission spectrometry.
(31) Lin, K.ꢀY. A.; Liu, Y.ꢀT.; Chen, S.ꢀY. J. Colloid Interface Sci.
2016, 461, 79ꢀ87.
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