Lewis acid mediated asymmetric [2,3]-sigmatropic rearrangement of allylic amines. Scope and mechanistic investigation
(Chemical Equation Presented) The first asymmetric [2,3]-sigmatropic rearrangement of achiral allylic amines has been realized by quaternization of the amines with an enantiomerically pure diazaborolidine and subsequent treatment with Et3N. The
Blid, Jan,Panknin, Olaf,Tuzina, Pavel,Somfai, Peter
p. 1294 - 1300
(2007/10/03)
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