18855-54-4Relevant academic research and scientific papers
Polyphosphine polyoxides as complexing agents of actinides for the removal from the nuclear wastes or from the human body
Cristau, Henri-Jean,Virieux, David,Pirat, Jean-Luc,Ansoborlo, Eric,Napoli, Marie Helene Henge,Paquet, Francois
, p. 505 - 508 (1999)
We synthesized two kinds of polyphosphine polyoxides. The first one has ether bridge and the second one shows PCP linkage. Complexation properties of these compounds towards minor actinides (Np, Pu and Am) have been evaluated from liquid-liquid extraction
Facile and general synthesis of polyphosphane polyoxides with (O)PCP(O) linkages
Cristau, Henri-Jean,Virieux, David,Mouchet, Patrick,Fruchier, Alain
, p. 1561 - 1569 (2007/10/03)
Polyphosphane polyoxides with (O)PCP(O) linkages are powerful chelating agents for extraction of actinides from nuclear wastes. They are obtained either by the Michaelis-Arbuzov reaction of chloromethylphosphane oxides and phosphorus(III) esters, or by the reaction of phosphane oxide carbanions with chlorophosphanes. With the latter method, the addition of a phosphane oxide carbanion in excess allowed us to overcome a transmetallation reaction and thereby obtain polyphosphane polyoxides in good yields. The 1H-NMR spectra of the PCH2P groups show the influence of the different R groups attached to the phosphorus atoms. We determined the coupling constants and the chemical shifts of these spin systems.
