189695-53-2Relevant academic research and scientific papers
Neutral and cationic monocarbonyl derivatives of palladium(II). X-ray crystal structure of [Pd(8-mq)(CO)(SPPh3)]ClO4
Ara, Irene,Fornies, Juan,Navarro, Rafael,Sicilia, Violeta,Urriolabeitia, Esteban P.
, p. 1963 - 1970 (2008/10/09)
Carbonylation of [Pd(8-mq)(OCMe2)x]ClO4 (8-mq = 8-quinolylmethyl-C,N) in CH2Cl2/Me2CO at low temperature gave [Pd(8-mq)(OClO3)(CO)]. Reactions of [Pd(8-mq)(OClO3)(CO)] with anionic (Cl-, Bi-, I-) or neutral (SPPh3, SPMe2Ph) nucleophiles in a 1 : 1 molar ratio resulted in the displacement of the weakly coordinated OClO3- group and the formation of the corresponding neutral [Pd(8-mq)(X)(CO)] (X = Cl, Br, I) or cationic [Pd(8-mq)(CO)L]ClO4 (L = SPPh3, SPMe2Ph) carbonyl complexes. The cationic complexes, [Pd(8-mq)(CO)L]ClO4, were synthesized by the reaction of [Pd(8-mq)(OCIO3)(SPPh3)] or [Pd(8-mq)(μ-SPMe2Ph)]2(ClO4)2 with CO. The X-ray structure of a cationic palladium carbonyl derivative, [Pd(8-mq) (CO)(SPPh3)]ClO4, is reported.
