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The complex [U(N(CH2CH2NSiMe2Bu(t))3)(η(1)-C=CC6H4-4-Me)] is a uranium alkynyl species featuring a bent U-C≡C unit (156°) and a triamidoamine ligand framework. It is derived from the protonolysis of a strained uranium metallacycle, demonstrating the reactivity of uranium complexes with carbon acids. The bent coordination geometry of the alkynyl ligand highlights the unique bonding interactions in uranium organometallic chemistry.

249284-53-5

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249284-53-5 Usage

Check Digit Verification of cas no

The CAS Registry Mumber 249284-53-5 includes 9 digits separated into 3 groups by hyphens. The first part of the number,starting from the left, has 6 digits, 2,4,9,2,8 and 4 respectively; the second part has 2 digits, 5 and 3 respectively.
Calculate Digit Verification of CAS Registry Number 249284-53:
(8*2)+(7*4)+(6*9)+(5*2)+(4*8)+(3*4)+(2*5)+(1*3)=165
165 % 10 = 5
So 249284-53-5 is a valid CAS Registry Number.

249284-53-5Downstream Products

249284-53-5Relevant academic research and scientific papers

Synthesis of a highly strained uranacycle: Molecular structures of organometallic products arising from reduction, oxidation and protonolysis

Boaretto, Rita,Roussel, Paul,Alcock, Nathaniel W.,Kingsley, Andrew J.,Munslow, Ian J.,Sanders, Christopher J.,Scott, Peter

, p. 174 - 184 (1999)

The reaction of [U(NN′3)I] [NN′3=N(CH2CH2NSiMe2Bu t)3] with Group 1 and 2 metal alkyls gives, via metalation of a methylsilyl group, a highly strained metallacycle [U(bit-NN′sub

Structure and reactions of a metallacyclic complex containing a remarkably long uranium-carbon bend

Boaretto, Rita,Roussel, Paul,Kingsley, Andrew J.,Munslow, Ian J.,Sanders, Christopher J.,Alcock, Nathaniel W.,Scott, Peter

, p. 1701 - 1702 (2007/10/03)

The intramolecular metalation of a β-silyl methyl group in [U{N(CH2CH2NSiMe2Bu(t))3}(CH2Ph)] occurs rapidly, despite the conformational demands of the triamidoamine ligand, to produce a highly strained metallacycle (U-C ca, 2.75 A); this complex reacts cleanly with a range of carbon and other acids to give, for example, an alkynyl with a bent (156°) U-C≡C unit.

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