Organic Letters p. 5489 - 5491 (2005)
Update date:2022-07-29
Topics:
Matharu, Daljit S.
Morris, David J.
Kawamoto, Aparecida M.
Clarkson, Guy J.
Wills, Martin
(Chemical Equation Presented) A rhodium(III) catalyst for asymmetric transfer hydrogenation of ketones has been designed. The incorporation of a tethering group between the diamino group and the cyclopentadienyl unit provides extra stereochemical rigidity. The catalyst is capable of enantioselective reduction of a range of ketones in excellent ee using formic acid/triethylamine as both the solvent and the reducing agent.
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