102493-46-9Relevant academic research and scientific papers
Some Molecular Hydrogen Complexes of Iridium
Crabtree, Robert H.,Lavin, Maryellen,Bonneviot, L.
, p. 4032 - 4037 (2007/10/02)
The new molecular hydrogen complexes + (bq = 7,8-benzoquinolinate, L = PPh3 or PCy3) and + are described.A 1H NMR T1 criterion is proposed for detecting such complexes.Deprotonation of the coordinated H2 is described.The mechanism of hydrogenolysis of d0 alkyls is discussed and a dihydrogen complex proposed as intermediate.
(1+) : A Non-classical Polyhydride Complex
Crabtree, Robert H.,Lavin, Maryellen
, p. 1661 - 1662 (2007/10/02)
(Cy = cyclohexyl) is shown by n.m.r. evidence, including T1 measurements, to undergo protonation to give the title complex, a bis(dihydrogen) dihydride, the first example of a non-classical polyhydride complex.
