7683-78-5Relevant academic research and scientific papers
Efficient synthesis of fumaric amides through cross-metathesis of acrylic amides with the NHC Grubbs ruthenium catalyst
Streuff, Jan,Mu?iz, Kilian
, p. 5973 - 5978 (2005)
Application of the second generation Grubbs metathesis catalyst for the homo-cross-metathesis of acroyl amides from chiral amines is reported. This efficient and high-yielding reaction provides a side-product free synthesis of fumaric acid diamides which
First asymmetric aminohydroxylation of acrylamides
Streuff, Jan,Osterath, Brigitte,Nieger, Martin,Muniz, Kilian
, p. 3492 - 3496 (2007/10/03)
The first examples of the asymmetric aminohydroxylation of acryl amides are reported. This was accomplished with chiral acrylamides as substrates, which undergo diastereoselective oxidative transformation within the so-called 'second catalytic cycle' with diastereomeric excesses reaching 100:0. The reaction relies solely on the stereochemical information provided by the enantiomerically pure starting materials. A stereochemical model for the observed asymmetric induction is provided.
