Chemical Communications p. 2333 - 2334 (1996)
Update date:2022-08-17
Topics:
Kelly, David R.
Knowles, Christopher J.
Mahdi, Jassem G.
Wright, Michael A.
Taylor, Ian N.
Roberts, Stanley M.
Wan, Peter W. H.
Grogan, Gideon
Pedragosa-Moreau, Sandrine
Willetts, Andrew J.
The enantiomeric bicyclic ketones 1, 3 and the tricyclic ketone 5 undergo stereochemically congruent Baeyer-Villiger oxidations with CHMO from Acinetobacter sp., CPMO from Pseudomonas sp. as well as 2,5-DKCMO, 3,6-DKCMO and MO2 from P. putida; in every case the tricyclic ketone 5 is transformed with > 96% ee. N-terminal sequences for the FAD/NADPH linked enzymes from Acinetobacter sp., Pseudomonas sp. and a novel CHMO from R. coprophilus have high homology with each other but no homology with the FMN/NADH linked enzymes; 2,5-DKCMO and 3,6-DKCMO.
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