Journal of the Chemical Society. Perkin transactions I p. 2659 - 2664 (1984)
Update date:2022-08-17
Topics:
Auret, Barbara J.
Balani, Suresh K.
Boyd, Derek R.
Greene, Ruth M. E.
Berchtold, Glenn A.
ortho-Hydroxylation of chloro- and bromo-benzene occurred in the presence of growing cultures of the fungi Rhizopus arrhizus, Rhizopus stolonifer, and Cunninghamella elegans.The absence of a primary kinetic isotope effect and the presence of the NIH shift are consistent with dihydroarene oxides being initial metabolites.N.m.r. analysis of the deuterium-labelled o-halogenophenol products suggested that enzyme-catalysed epoxidation occurs preferentially at the 2,3-bond.
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