Journal of the Chemical Society. Chemical communications p. 1897 - 1898 (1994)
Update date:2022-08-17
Topics:
Djurovich, Peter I.
Dolich, Alfred R.
Berry, Donald H.
Four-legged piano stool complexes (η6-arene)Ru(H)2(SiEt3)2 and (η5-C5Me5)Rh(H)2(SiEt3)2 catalyse the transfer dehydrogenative coupling of Et3SiH in the presence of a hydrogen acceptor such as tert-butylethylene to yield the carbosilane dimer, HSiEt2CHMeSiEt3, and 2,2-dimethylbutane by a mechanism involving an intermediate η2-silene complex, LnM(Et2Si=CHMe), generated by β-hydrogen elimination from a silyl group.
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