C-H bond cleavage in uranium(III) thiolato complexes can occur via oxidative addition reactions. This involves the insertion of the uranium atom into the C-H bond to form new uranium-carbon and uranium-hydrogen bonds. This process is typically associated with a change in the oxidation state of uranium. Mechanistically, C-H bond cleavage in uranium(III) thiolato complexes may involve the transfer of a hydrogen atom from the C-H bond to the uranium center, leading to the formation of a U(IV) species. These reactions can be catalytic in nature, where the uranium(III) complex acts as a catalyst for C-H activation and functionalization reactions. This can have implications in organic synthesis and hydrocarbon activation processes.
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N,N-diethyl-4-cyanobenzenesulfonamide
2-((dimethylamino)methyl)-5-iodophenol
(E)-2-(2-(4-methylstyryl)phenyl)propan-2-amine
