Angewandte Chemie - International Edition p. 3694 - 3698 (2017)
Update date:2022-08-04
Topics:
Yang, Qi
Zhang, Long
Ye, Chen
Luo, Sanzhong
Wu, Li-Zhu
Tung, Chen-Ho
Reported herein is an unprecedented photocatalytic asymmetric cross-dehydrogenative coupling reaction between tertiary amines and simple ketones, and it proceeds by synergistic multiple catalysis with substoichiometric amounts of a hydrogen acceptor. This process is enabled by a simple chiral primary amine catalyst through the coupling of a catalytic enamine intermediate and an iminium cation intermediate in situ generated from tetrahydroisoquinoline derivatives by coupled Ru/Co catalysis.
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