Angewandte Chemie - International Edition in English p. 1183 - 1185 (1997)
Update date:2022-08-17
Topics:
Ooi
Kondo
Maruoka
Success at last: The 1,4-allylation of α,β-unsaturated aldehydes with selectivities up to 95/5 and yields of 83% has been achieved thanks to the newly developed Lewis acidic receptor p-F-ATPH (L= 2,6-(p-FC6H4)2C6H3O). In addition to a coordination site for the aldehyde, this possesses an appropriate coordination site for a reactive nucleophile, as shown schematically on the right.
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Doi:10.1021/jacs.5b08535
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(1970)Doi:10.1021/ja01568a042
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(1927)Doi:10.1002/anie.201403885
(2014)Doi:10.1016/S0040-4039(00)78990-8
(1980)
