Spectrochimica Acta Part A: Molecular and Biomolecular Spectroscopy p. 1187 - 1190 (1993)
Update date:2022-08-17
Topics:
Kubozono, Y.
Miyamoto, T.
Shinmyozu, T.
Aoyagi, M.
Gondo, Y.
et al.
The radical cations of butatriene (BT+.) and tetramethylbutatriene (TMBT+.) have been stabilized in low-temperature halocarbon matrices studied by ESR spectroscopy.The spectra of BT+. and TMBT+. exhibit isotropic hyperfine splittings of 8.3 G (4H) and 13.0 G (12H), respectively.The skew angles of BT+. (25 deg) and TMBT+. (50 deg) are estimated by comparison the experimental hyperfine splittings with those obtained by semiempirical MO calculations.
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