22228-41-7Relevant academic research and scientific papers
Cyanohydrin-Mediated Cyanation of Remote Unactivated C(sp3)-H Bonds
Wang, Min,Huan, Leitao,Zhu, Chen
, p. 821 - 825 (2019)
A new approach for generation of alkoxy radical from the O-H bond of cyanohydrin promoted by visible-light photoredox catalysis is reported. The alkoxy radical triggers the successive remote HAT and intramolecular cyano migration, leading to the regiosele
Nickel-Catalyzed C(sp3)-H Functionalization of Benzyl Nitriles: Direct Michael Addition to Terminal Vinyl Ketones
Zhang, Ninghui,Zhang, Chunli,Hu, Xiaoping,Xie, Xin,Liu, Yuanhong
, p. 6004 - 6009 (2021/07/31)
An efficient nickel(0)-catalyzed addition of benzyl nitriles to terminal vinyl ketones via C(sp3)-H functionalization has been developed. The reaction provides a novel and efficient protocol for the synthesis of α-functionalized benzyl nitriles with a wide range of structural diversity under mild reaction conditions while obviating the use of a strong base. The work might be potentially useful toward the development of an enantioselective variant using chiral nitrogen ligands.
Visible-light-induced triple catalysis for a ring-opening cyanation of cyclopropyl ketones
Liu, Jing,Liu, Xiao-Peng,Wu, Hong,Wei, Yi,Lu, Fu-Dong,Guo, Kai-Rui,Cheng, Ying,Xiao, Wen-Jing
supporting information, p. 11508 - 11511 (2020/10/12)
An unprecedented triple catalytic, general ring-opening cyanation reaction of cyclopropyl ketones for the construction of γ-cyanoketones is described. The key is to merge photoredox catalysis with Lewis acid catalysis and copper catalysis to enable the selective cleavage of the carbon-carbon bonds and the selective coupling of the generated radical and cyanide anion.
