Chemical Communications p. 11508 - 11511 (2020)
Update date:2022-08-04
Topics:
Liu, Jing
Liu, Xiao-Peng
Wu, Hong
Wei, Yi
Lu, Fu-Dong
Guo, Kai-Rui
Cheng, Ying
Xiao, Wen-Jing
An unprecedented triple catalytic, general ring-opening cyanation reaction of cyclopropyl ketones for the construction of γ-cyanoketones is described. The key is to merge photoredox catalysis with Lewis acid catalysis and copper catalysis to enable the selective cleavage of the carbon-carbon bonds and the selective coupling of the generated radical and cyanide anion.
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