Tetrahedron p. 8419 - 8430 (1992)
Update date:2022-08-05
Topics:
Faure
Pommier
Pons
Rajzmann
Santelli
Friedel-Crafts acylation of alkenes with β,γ-alkenoyl halides leads to conjugated Al-trienolates able to cyclize into Al-enolates of 2-cyclohexenones through an allowed thermal disrotary electrocyclization mechanism. Discussion of the product structures is based on two-dimensional NMR experiments (400 MHz) and molecular mechanics studies (GENMOL and MM2).
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