Bulletin of the Chemical Society of Japan p. 347 - 352 (1990)
Update date:2022-08-05
Topics:
Bonazzola
Michaut
Roncin
Misawa
Sakuragi
Tokumaru
γ-Irradiation of phenyl-and diphenylethenes in CFCl3 matrix at 77 K resulted in the formation of the substrate radical cations. 1,1-Diphenyl-2-methylpropene radical cations exhibit a spin density (ρ=0.45) at the β carbon much higher than those of stilbene and 2-styrylnaphthalene radical cations and comparable to those of styrene and α-methylstyrene radical cations. The spin density at the vinyl carbons appears to play an important role in governing the reactivity of the olefin radical cations with molecular oxygen.
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