Journal of the Chemical Society. Chemical communications p. 1405 - 1408 (1990)
Update date:2022-08-10
Topics:
Umezawa, Toshiaki
Davin, Laurence B.
Yamamoto, Etsuo
Kingston, David G. I.
Lewis, Norman G.
Both (+)-pinoresinol 6a in Forsythia suspensa and (-)-secoisolariciresinol 14a in F. intermedia are formed via a direct stereochemically-controlled coupling of coniferyl alcohol 2 derived moieties (cf. the typical peroxidase-catalysed reaction in the presence of H2O2), and the dibenzylbutyrolactone lignan, (-)-matairesinol 10a, in F. intermedia is formed from a post-coupling modification of (-)-secoisolariciresinol 14a; this transformation has been demonstrated in vivo, and in vitro with a crude enzyme preparation, and represents the first report of an enzyme specifically involved in lignan biosynthesis.
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