Catalysis Letters p. 1832 - 1838 (2014)
Update date:2022-08-22
Topics:
Bachrach, Mark
Morlanes-Sanchez, Natalia
Canlas, Christian P.
Miller, Jeffrey T.
Marks, Tobin J.
Notestein, Justin M.
Catalysts consisting of Pd nanoparticles supported on highly dispersed TiOx-Al2O3, TaOx-Al2O3, and MoOx-Al2O3 are studied for catalytic quinoline hydrogenation and selective C-N bond cleavage at 275°C and 20 bar H2. The Pd/MOx-Al2O3 materials exhibit significantly greater aromatic product selectivity and thus 10-15 % less required H2 for a given level of denitrogenation relative to an unmodified Pd/Al2O3 catalyst.
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