Journal of the American Chemical Society p. 822 - 826 (1985)
Update date:2022-08-17
Topics:
Friedman, Ronald S.
Andrews, Lester
Matrix photoionization experiments with o- and m-dichlorobenzene and 1,2,4-trichlorobenzene produced and isolated for spectroscopic study not only radical cations of the precursor compound but also rearranged cation products.It is postulated that a bridged chloronium ions is formed upon excitation to the lone pair hole state which serves as an intermediate in rearrangements among the excited-state di- and trichlorobenzene cation isomers.The chlorine lone pair hole excited state facilitates a "chloronium ion walk" around the aromatic ring.
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Doi:10.1007/BF00515425
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