Angewandte Chemie - International Edition p. 1859 - 1863 (2017)
Update date:2022-08-05
Topics:
Sarria Toro, Juan M.
García-Morales, Cristina
Raducan, Mihai
Smirnova, Ekaterina S.
Echavarren, Antonio M.
Chloromethylgold(I) complexes of phosphine, phosphite, and N-heterocyclic carbene ligands are easily synthesized by reaction of trimethylsilyldiazomethane with the corresponding gold chloride precursors. Activation of these gold(I) carbenoids with a variety of chloride scavengers promotes reactivity typical of metallocarbenes in solution, namely homocoupling to ethylene, olefin cyclopropanation, and Buchner ring expansion of benzene.
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