Organic Letters p. 6333 - 6336 (2019)
Update date:2022-09-26
Topics:
Zou, Suchen
Gao, Bao
Huang, Yao
Zhang, Tianze
Huang, Hanmin
A novel and atom-economic palladium-catalyzed isomerization-hydrocarbonylative cyclization reaction of 1,5-dienes to 2-alkylidenecyclopentanones has been developed, which provides a rapid and straightforward approach to 2-alkylidenecyclopentanones with high stereoselectivity. The reaction was found to proceed via alkene isomerization and selective hydrocarbonylative cyclization to generate 2-alkylidenecyclopentanones with high selectivity.
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