Chemistry - A European Journal p. 9911 - 9914 (2011)
Update date:2022-07-30
Topics:
Zhao, Qiwu
Curran, Dennis P.
Malacria, Max
Fensterbank, Louis
Goddard, Jean-Philippe
Lacote, Emmanuel
Reducing alkenes to tears: Addition of structurally diverse N-heterocyclic carbenes (NHCs) to silicon allows the reduction of propargylic and styryl alcohols through an organocatalyzed silylation/direct hydride transfer tandem reaction (see scheme). Catalytic turnover is enabled by the switch to and from hypervalent silicon. This provides a new synthetic application of NHC-main group element complexes. Copyright
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