Journal of the American Chemical Society p. 18944 - 18947 (2012)
Update date:2022-08-04
Topics:
Trost, Barry M.
Kaneko, Toshiyuki
Andersen, Neil G.
Tappertzhofen, Christoph
Fahr, Bruce
The first total synthesis of aeruginosin 98B was accomplished. The key step is a highly diastereoselective Pd-catalyzed intramolecular asymmetric allylic alkylation reaction of a diastereomeric mixture of allylic carbonates that is enabled by the use of racemic phosphine ligand L1.
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