Journal of the American Chemical Society p. 11430 - 11434 (2019)
Update date:2022-08-04
Topics:
Ghorai, Samir
Chirke, Sahadev Shrihari
Xu, Wen-Bin
Chen, Jia-Feng
Li, Changkun
The first earth-abundant cobalt-catalyzed highly branched- and enantioselective allylic amination of racemic branched allylic carbonates bearing alkyl groups with both aromatic and aliphatic amines has been developed. The process allows rapid access of allylic amines in high yields with exclusively branched selectivity and excellent enantioselectivities (normally 99% ee) under mild reaction conditions.
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