Tetrahedron p. 7959 - 7980 (1995)
Update date:2022-07-29
Topics:
Bowman, W. Russell
Stephenson, Peter T.
Terrett, Nicholas K.
Young, Adrian R.
Radical cyclisation of sp3 carbon-centred radicals onto imines and hydrazones provides a new method for the synthesis of 5- and 6-membered ring nitrogen heterocycles. Cyclisation onto the electrophilic carbon of the C=N group and 5-exo stereoelectronic selectivity are the dominating mechanistic parameters. The C-centred radical intermediates were generated from benzeneselenyl precursors using Bu3SnH.
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