Tetrahedron p. 12197 - 12214 (1998)
Update date:2022-09-26
Topics:
Morimoto, Yoshiki
Yokoe, Chiho
Kurihara, Hajime
Kinoshita, Takamasa
The total syntheses of haliclamines A (1) and B (2), macrocyclic marine alkaloids closely related to the key bisdihydropyridine intermediate 3 of the biogenetically unique manzamine family, have efficiently been achieved via stepwise controlled inter- and intramolecular N-alkylations of 3- alkylpyridine derivatives such as 40 and 41. The general synthetic methodology toward the bispyridinium macrocycle 44, a key biogenetic equivalent of the polycyclic marine alkaloids, has been proposed through the total syntheses.
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Doi:10.1081/SCC-120020209
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(1998)Doi:10.1055/s-2007-982539
(2007)Doi:10.1023/A:1010427928327
(2001)Doi:10.1080/00397919808005076
(1998)Doi:10.1007/pl00010155
(1998)