Organic Letters p. 4166 - 4169 (2016)
Update date:2022-08-05
Topics:
Luo, Bo
Gao, Jin-Ming
Lautens, Mark
A palladium-catalyzed, norbornene-mediated tandem amination/cyanation reaction via Catellani-type C-H functionalization was developed using N-benzoyloxyamines as the amination reagent and Zn(CN)2 as the terminating agent. This transformation, in which one C-N bond and one C-C bond are formed, provides an efficient approach for the synthesis of ortho-aminated benzonitriles in one pot from easily accessible starting materials.
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