Bioorganic and Medicinal Chemistry p. 821 - 824 (1996)
Update date:2022-08-10
Topics:
Hage
Schnelten
Sawyer
Several iron(II) complexes [Fe(II)L(x); Fe(II)(DPAH)2 (DPAH2 = 2,6- dicarboxyl pyridine), Fe(II)(PA)2 (PAH = picolinic acid) and Fe(II)(bpy)2/2+ (bpy = 2,2'-bipyridine)] in combination with a reductant [DH2; PhNHNHPh (mimic of dihydroflavin)] catalytically activate O2 (1 atm) for the demethylation of N-methylanilines [PhN(CH3)2, PhNH(CH3)]. This chemistry, which appears to involve a Fenton-like intermediate [L(x)Fe(IV)OOH(DH) (1c)], mimics that of the cytochrome P-450 monooxygenase/reductase proteins.
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