Journal of the Chemical Society. Chemical communications p. 851 - 853 (1982)
Update date:2022-08-29
Topics:
Symons, Martyn C. R.
McConnachie, Glen D. G.
The 1H hyperfine coupling for Me3P.+ ions generated radiolytically in Freon at 77 K (ca. 11.5 G) is much greater than that for the dimer cations (Me3P)2+ (ca. 3.3 G): this is explained in terms of a decreasing tendency for ?-? delocalisation as the pyramidal character of the Me3P unit increases, coupled with a tendency towards ?-orbital localisation in ?*-radicals.
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