Journal of the American Chemical Society p. 1404 - 1408 (1986)
Update date:2022-08-16
Topics:
Knight, J. S.
Freeman, C. G.
McEwan, M. J.
The relative proton affinities of CH3CN (acetonitrile) and CH3NC (methyl isocyanide were determined by using the Selected Ion Flow Tube technique.Two distinct species were observed for the C2H4N+ ion: one produced from CH3CN and one from CH3NC.The two C2H4N+ isomers were readily distinguished in the flow tube by their different reactivity.The association product, C2H4N+, of the ion-molecule reaction between CH3+ and HCN was shown to be present in both isomeric forms in the ratio 85percent protonated acetonitrile and 15percent protonated methyl isocyanide.
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