Journal of the Chemical Society - Faraday Transactions p. 2907 - 2912 (1991)
Update date:2022-08-10
Topics:
Hanning-Lee, Mark A.
Pilling, Michael J.
Warr, Jonathan F.
A time-resolved study has been performed at conditions close to criticality in the H2-O2 system.Reaction was initiatd by the exciplex laser flash photolysis of O2 at 193.3 nm.H was monitored using time-resolved resonance fluorescence and showed an approximately biexponential time dependence.Near the explosion limit, the long-time behaviour is dominated by the competition between the branching and terminating H + O2 channels.Rate coefficients for these channels were inferred from this time dependence over the ranges 800 <*> T/K <*> 850 and 100 <*> P/Torr <*> 243.
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