The influence of porosity and active sites of zeolites Y and beta on the co-cracking of n-decane and 2-Ethylphenol (cas 90-00-6)

Add time:07/12/2019    Source:sciencedirect.com

We investigated the cracking of n-decane and 2-ethylphenol as co-substrate in a 90/10 wt.-% mixture over zeolites Y and beta. The use of these substrates aimed to better understand the occurring chemistry in applications such as Co-FCC. We employed a number of different zeolites Y with different amounts of active sites and pore volumes. Additionally, the pore system of zeolite beta was modified by basic leaching. The materials were characterized by N2 physisorption, ICP-OES, XRD, 27Al, 1H, 13C MAS NMR, NH3-TPD, IR and TGA. It was found that the activity of the catalysts depends on the number of Brønsted acid sites as determined by NMR spectroscopy. Also most important is the mesopore volume/mesopore surface which is beneficial for the diffusion towards the micropores, especially for zeolite Y that is able to deoxygenate phenols.

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