Deuterium permeation behavior in iron-irradiated erbium oxide (cas 12645-29-3) coating

Add time:07/23/2019    Source:sciencedirect.com

Tritium permeation barrier has been developed for mitigating fuel loss and radiological concern at a fuel breeding/recovery system in a D-T fusion reactor. Recent research effort has been dedicated to erbium oxide (cas 12645-29-3) coatings, and various hydrogen permeation behaviors except for irradiation effects have been elucidated. In this study, irradiation effects on deuterium permeation through erbium oxide coatings have been investigated by iron-ion irradiation at elevated temperature followed by deuterium gas-driven permeation experiments. The coatings deposited on reduced activation ferritic steel substrates with displacement damages of 0.01–1 dpa showed one or two orders of magnitude different permeabilities at 300–500 °C; however, the permeabilities became comparable and lower than that of unirradiated at 550–700 °C, indicating the grain growth and the formation of grain boundaries with a lower permeability. Cross-sectional transmission electron microscopy with selected-area electron diffraction for the coatings before and after the permeation experiments indicated the formation of a defect-accumulated region. The stability of the region strongly depends on the irradiation condition: damage concentration and annealing time, resulting in the difference of the permeability and diffusivity in the lower temperature range.

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