Picosecond studies of jet-cooled Chromyl chloride (cas 14977-61-8)

Add time:07/17/2019    Source:sciencedirect.com

The dynamics of the 1B1 state of chromyl chloride, CrO2Cl2, are investigated via picosecond time-resolved measurements on a jet-cooled sample. Quasi-biexponential time evolution of fluorescence is observed for each of the nine single vibronic levels studied. A rapid, mode-dependent acceleration of the decay rates with excess vibrational energy is reported. The time dependence is described by a kinetic model and the non-radiative decay channels which may be responsible for the observed behavior are discussed.

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