Organic Letters p. 2035 - 2037 (2008)
Update date:2022-08-02
Topics:
Akagawa, Kengo
Akabane, Hajime
Sakamoto, Seiji
Kudo, Kazuaki
A resin-supported N-terminal prolyl peptide having a β-turn motif and hydrophobic polyleucine chain effectively catalyzed the asymmetric transfer hydrogenation under aqueous conditions. The polyleucine tether provides a hydrophobic cavity in aqueous media that brought about a remarkable acceleration of the reaction. In addition, the polyleucine chain also turned out to be essential for high enantioselectivity.
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