Organic Letters p. 488 - 492 (2020)
Update date:2022-08-02
Topics:
Deng, Zhi-Xiong
Zheng, Yu
Xie, Zhen-Zhen
Gao, Yue-Heng
Xiao, Jun-An
Xie, Si-Qi
Xiang, Hao-Yue
Chen, Xiao-Qing
Yang, Hua
We herein report a phosphine-mediated domino process of MBH-Type reaction/umpolung γ-Addition through the rational integration of the privileged reactivities of alkynoate. Simply by manipulating the nucleophilic reagent, the developed protocol offers a facile, diversity-oriented construction of a wide range of three-substituted coumarins.
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