Chemical Communications p. 14021 - 14024 (2018)
Update date:2022-08-04
Topics:
Cera, Gianpiero
Lanzi, Matteo
Bigi, Franca
Maggi, Raimondo
Malacria, Max
Maestri, Giovanni
An in situ formed palladium hydride catalyst enables the sequential dual isomerization of propargylamide derivatives to 1-amido-1,3-dienes with high chemo- and regioselectivity. The reaction shows ample functional group tolerance, delivering a valuable class of products, including highly deuterated ones, from readily available reagents. The reaction occurs through a complex mechanism studied by DFT modelling.
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(2021)
