The First Molecular Electronic Hyperpolarizabilities of Highly Polarizable Organic Molecules: 2,6-Di-tert-butylindoanilines

DOI: 10.1039/c39920000672

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Journal of the Chemical Society. Chemical communications p. 672 - 674 (1992)

Update date:2022-08-06

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Authors:

Marder, Seth R.

Cheng, Lap-Tak

Tiemann, Bruce G.

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Article abstract of DOI:10.1039/c39920000672

The first molecular hyperpolarizabilities (β) of series of 2,6-di-tert-butylindoanilines, measured by electric-field-induced second harmonic generation, are somewhat more sensitive to donor strengh than was found for analogously substituted nitrostilbenes, and dimethylindoaniline has a β roughly twice that of its 2,6-di-tert-butylated analogue, measured in chloroform; solvatochromic measurements on the former compound suggest that that this decrease in hyperpolarizability is consistent with a bound-solvent effect.

Full text of DOI:10.1039/c39920000672

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