Chemistry - A European Journal p. 16292 - 16296 (2012)
Update date:2022-08-05
Topics:
Peng, Bo
O'Donovan, Daniel H.
Jurberg, Igor D.
Maulide, Nuno
Rearranging its feathers: The transformation of simple linear amides into a diverse range of branched, functionalized products by conversion to iminium esters is followed by sequential treatment with nucleophiles and electrophiles (see scheme). The method takes advantage of a novel Claisen rearrangement and the use of aromatic substrates greatly facilitates the formation of the intermediate iminium ether.
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