Organic Letters p. 6461 - 6465 (2021)
Update date:2022-08-02
Topics:
Zhou, You
Zhao, Peng
Wang, Li-Sheng
Yu, Xiao-Xiao
Huang, Chun
Wu, Yan-Dong
Wu, An-Xin
A novel [2 + 1 + 3] cyclization reaction for the synthesis of 2-aryl-4-quinolinecarboxylates from aryl methyl ketones, arylamines, and 1,3-dicarbonyl compounds has been established. This metal-free process achieved the C-C bond cleavage of 1,3-dicarbonyl compounds directly as a single-carbon synthon. The reaction is highly efficient and has good substrate compatibility while operating under mild conditions. This method has good practicability and successfully realized the synthesis of bioactive molecules.
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