Tetrahedron Letters p. 4443 - 4444 (1999)
Update date:2022-07-29
Topics:
Harrowven, David C.
Lucas, Matthew C.
Howes, Peter D.
Total syntheses of two marine sesquiterpenes, aplysin 1 and debromoaplysin 2, are described. The key step involves a diastereoselective, sulfur mediated radical cyclisation of diene 5 to 7 which simultaneously creates the sterically demanding aplysin skeleton and establishes the relative configuration of the three contiguous stereogenic centres.
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Doi:10.1055/s-1999-2629
(1999)Doi:10.1007/BF00938248
(1969)Doi:10.1016/S0040-4039(98)02637-9
(1999)Doi:10.1016/S0957-4166(98)00466-2
(1999)Doi:10.1039/b316099h
(2004)Doi:10.1016/S0960-894X(99)00068-2
(1999)
