Beilstein J. Org. Chem. 2017, 13, 384–392.
4. Terao, J.; Kambe, N. Acc. Chem. Res. 2008, 41, 1545.
of any one of the alkenes from this structure would lead to anti-
bonding relationships to bond to the alpha carbon.
5. Martin, R.; Buchwald, S. L. Acc. Chem. Res. 2008, 41, 1461.
Conclusion
6. Marion, N.; Nolan, S. P. Acc. Chem. Res. 2008, 41, 1440.
In summary, we present information that is of value to
advancing the area of metal-catalyzed decarboxylative coupling
reactions, specifically those of pentadienyl dienoates that do not
require an anion-stabilizing group, are run at ambient tempera-
ture, and can utilize the more accessible alcohol for a leaving
group. This reaction was advanced to be possible in a two-com-
ponent fashion, allowing for the conversion of dienoic acids and
pentadienyl alcohols into 1,3,6,8-tetraenes with the only stoi-
chiometric byproducts being water and carbon dioxide. These
reactions currently require a diene motif with each coupling
partner, but the product maintains the independent reactivity op-
portunities of these isolated dienes as opposed to forming the
fully conjugated 1,3,5,7-tetraene. A variety of substrates were
explored where each of the unique positions on the coupling
partners was modified and two different mechanistic pathways
are presented. A more in-depth mechanistic analysis to improve
the yields and to explore other reactivity possibilities based on
this process are currently being studied and will be published in
due time.
7. Denmark, S. E.; Regens, C. S. Acc. Chem. Res. 2008, 41, 1486.
8. Kantchev, E. A. B.; O'Brien, C. J.; Organ, M. G. Angew. Chem., Int. Ed.
9. Corbet, J.-P.; Mignani, G. Chem. Rev. 2006, 106, 2651.
10.Schaub, T. A.; Kivala, M. Cross-Coupling Reactions to sp Carbon
Atoms. Metal-Catalyzed Cross-Coupling Reactions and More;
Wiley-VCH Verlag GmbH & Co. KGaA: Weinheim, 2014; pp 665 ff.
11.Davies, H. M. L.; Morton, D. J. Org. Chem. 2016, 81, 343.
12.Brückl, T.; Baxter, R. D.; Ishihara, Y.; Baran, P. S. Acc. Chem. Res.
13.Stuart, D. R.; Fagnou, K. The Discovery and Development of a
Palladium(II)-Catalyzed Oxidative Cross-Coupling of Two Unactivated
Arenes. In Inventing Reactions; Gooßen, L. J., Ed.; Springer: Berlin,
Heidelberg, 2013; pp 91 ff.
14.Colby, D. A.; Bergman, R. G.; Ellman, J. A. Chem. Rev. 2010, 110,
15.Campeau, L.-C.; Rousseaux, S.; Fagnou, K. J. Am. Chem. Soc. 2005,
16.Stuart, D. R.; Alsabeh, P.; Kuhn, M.; Fagnou, K. J. Am. Chem. Soc.
17.Gorelsky, S. I.; Lapointe, D.; Fagnou, K. J. Org. Chem. 2012, 77, 658.
Supporting Information
18.Lafrance, M.; Fagnou, K. J. Am. Chem. Soc. 2006, 128, 16496.
Supporting Information File 1
Experimental procedures and analytical data for all
substrates and products, product inhibition study,
computational calculation information, and relevant
energies and Cartesian coordinates.
19.Jana, R.; Trivedi, R.; Tunge, J. A. Org. Lett. 2009, 11, 3434.
20.Tokoroyama, T.; Nakamura, M. Chem. Lett. 1977, 6, 659.
21.Tsuda, T.; Chujo, Y.; Nishi, S.; Tawara, K.; Saegusa, T.
22.Tsuda, T.; Okada, M.; Nishi, S.; Saegusa, T. J. Org. Chem. 1986, 51,
23.Trost, B. M.; Bunt, R. C. J. Am. Chem. Soc. 1998, 120, 70.
Acknowledgements
Funding for this project from the North Carolina Biotech-
nology Center (BRG-1205) and University of North Carolina at
Greensboro is gratefully acknowledged. The authors thank Dr.
Franklin J. Moy for assisting with analysis of NMR data and
Dr. Daniel A. Todd for acquisition of the high resolution mass
spectrometry data at the Triad Mass Spectrometry Laboratory at
the University of North Carolina at Greensboro.
24.Corey, E. J.; Fraenkel, G. J. Am. Chem. Soc. 1953, 75, 1168.
25.Waetzig, S. R.; Rayabarapu, D. K.; Weaver, J. D.; Tunge, J. A.
26.Waetzig, S. R.; Tunge, J. A. J. Am. Chem. Soc. 2007, 129, 14860.
27.Grenning, A. J.; Tunge, J. A. Org. Lett. 2010, 12, 740.
28.Rayabarapu, D. K.; Tunge, J. A. J. Am. Chem. Soc. 2005, 127, 13510.
References
29.Sim, S. H.; Park, H.-J.; Lee, S. I.; Chung, Y. K. Org. Lett. 2008, 10,
1. Torborg, C.; Beller, M. Adv. Synth. Catal. 2009, 351, 3027.
30.Pi, S.-F.; Tang, B.-X.; Li, J.-H.; Liu, Y.-L.; Liang, Y. Org. Lett. 2009, 11,
2. McGlacken, G. P.; Fairlamb, I. J. S. Eur. J. Org. Chem. 2009, 4011.
31.Torregrosa, R. R. P.; Ariyarathna, Y.; Chattopadhyay, K.; Tunge, J. A.
3. Nicolaou, K. C.; Bulger, P. G.; Sarlah, D. Angew. Chem., Int. Ed. 2005,
391