Bulletin of the Chemical Society of Japan p. 1235 - 1242 (1991)
Update date:2022-08-06
Topics:
Eiki, Toshio
Tagaki, Waichiro
Effects of various metal ions on the methanolysis of phenyl phosphatosulfate having P-O-S linkage were investigated.Metal ions examined were found to be divided into two different groups in the manner of cleavage of P-O-S linkage: Mg2+, Cr3+, Cu2+, Mn2+, and Ca2+ with larger ionic radii catalyzed the selective P-O bond cleavage, while Be2+, Al3+, Fe2+, And Zn2+ with smaller ionic radii promoted the selective S-O bond cleavage.Such selectivity was discussed in terms of the difference in the mechanism of P-O and S-O bond cleavage.
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