Tetrahedron Letters p. 5820 - 5824 (2016)
Update date:2022-08-10
Topics:
Xie, Fukai
Du, Chuan
Pang, Yadong
Lian, Xu
Xue, Chentao
Chen, Yanyu
Wang, Xuefei
Cheng, Maosheng
Guo, Chun
Lin, Bin
Liu, Yongxiang
A microwave-assisted N-fluorobenzenesulfonimide (NFSI)/Lewis acid-catalyzed Beckmann rearrangement was developed. The remarkable promotion to the electrophilicity of NFSI by Lewis acids was illustrated utilizing a series of readily available oxime substrates. The action model between NFSI and Lewis acids was probed by control experiments and theoretical calculations.
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