Chemistry Letters p. 763 - 766 (1985)
Update date:2022-08-11
Topics:
Ballantine, James A.
Jones, William
Purnell, J. Howard
Tennakoon, Dayananda T. B.
Thomas, John M.
Evidence is provided for two alternative pathways for the reactions undergone by 2-methylpropene between the layers of a sheet silicate catalyst (Al3+-exchanged montmorillonite).This clay, when it initially contains ca. 12percent interlayer water, catalyses the addition of either water or methanol to 2-methylpropene to yield, respectively, t-butanol or 2-methoxy-2-methyl propane (methyl tertiary butyl ether, MTBE), whereas the same clay following deliberate dehydration acts as an effective catalyst for the oligomerisation of 2-methylpropene.Similar results are obtained with an Al3+-exchanged synthetic hectorite.
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