Tetrahedron Letters p. 6009 - 6012 (1999)
Update date:2022-08-23
Topics:
Pale-Grosdemange, Catherine
Merkofer, Thorsten
Rohmer, Michel
Poralla, Karl
Mutagenesis of Tyr420 to Ala in the catalytic cavity of squalene-hopene cyclase of Alicyclobacillus acidocaldarius resulted in an altered product spectrum. Besides hopene and diplopterol, this mutant produced significant amounts of the bicyclic α- and γ-polypodatetraenes and minor amounts of the tricyclic 13α(H)-malabaricatriene.
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