Bulletin of the Chemical Society of Japan p. 2040 - 2045 (1984)
Update date:2022-08-12
Topics:
Ishikawa
Arai
CO//2 TEA laser-induced photolysis of C//2H//5F was studied by using a time-resolved infrared fluorescence technique. Molecular elimination of vibrationally excited hydrogen fluoride (HF*) from C//2H//5F*** occurs in the process. Rotational temperatures and vibrational level populations of HF* are estimated from observed fluorescence spectra by computational fitting. Higher vibrational level are populated to a less extent in the decomposition under a collisionless condition. When the pressure of C//2H//5F is increased, however, population inversion is allowed among some levels. Possible reaction mechanism is discussed for the production of HF* at extraordinarily high vibrational levels.
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